In "Peewit's Unscrupulous Adventure," Jokey Smurf used one of his explosive presents to stop some mooks.
There's a moment for Gargamel in the opening credits, using footage taken from a special episode from the previous season of the show
Gargamel:(with Power Echoes while standing on a mountain) Ravage the land as never before! / Total destruction FROM MOUNTAIN TO SHORE!
In "The Purple Smurfs", Papa Smurf needed one of the titular Smurfs every time he had a possible cure for The Virus causing the transformation, something not easy due the purplified Smurfs becoming stronger under its effects and Hefty being the second Purple Smurf. In the second attempt, the three Smurfs who Got Volunteered managed to overpower and bring him Smurfin' Hefty.
Clumsy, gets special mention later in the film. Throughout the film, he's stayed at the Winslow home with Grace while the other smurfs looked for a stargazer, and later the spell they need. But, after he finds out Papa Smurf has been captured by Gargamel. Gutsy and the other smurfs tell Clumsy and the Winslows that Papa told them to save themselves. Clumsy, says "No, we can't leave Papa behind!" and "No, No, No We can't!" He then tells, "There is no way, we're leaving without Papa."
Later, Brainy says the incantation, which opens the portal to Smurf Village. Then, Gargamel heads outside and hears Grouchy, Clumsy and Brainy saying.
Grouchy: You have our Papa, prepared to get Smurfed.
Clumsy: Yeah, what he said.
Brainy: Hey Gargamel, make that three little smurfs. (lights up a firework signaling the other smurfs to come out) And, I went home and brought a few friends!