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Fred_H
Since: May, 2013
2013-06-05 04:57:52
I don't know anything about anime (or very much about Japanese), but it says "ふたりのきもちのほんとのひみつ" right there in the video. Google translates this as "the secret of the truth of the feelings of Two", and the first hit
for the title says it is
the ending theme song of the TV anime "Kill Me Babe!".
Does that help?
EDIT: Here's the (English) Wikipedia page
for the anime.
Zanreo
(Ten years in the joint)

Does anyone know what song 27 here is: https://www.youtube.com/watch?v=sQLsEJc_Vn8
(go to 3:48 to hear it)
I KNOW I've heard it before, but I can't remember where I heard it before or what it was called... I think it might have been a Vocaloid song, or music from an anime/game, but I'm not completely sure.