Crowning Moment of Funny: "When he later finished his research project, it said 'There are wild rhinos and lions roaming around in Japan.' It provoked sharp criticism, but that is a different story..."
The ending of Shiina's fight with Shishido. "RABBIT BITCH-SLAP!" Then he gets it into his head that maybe he'll turn back into a human if he does it repeatedly.
Crowning Moment of Heartwarming: The aforementioned Crowning Moment of Awesome for Kasai. Then there's the ending of the aquarium arc, where Aoi Hana is thinking about how the reason Shiina is turning back to normal while Isana wasn't was because Shiina was also bonding with the zoo animals instead of treating them badly. She then turns to Shiina and asks him if they can keep having fun while making the zoo popular. Shiina's response is to grin and say "That's a given!"